Bulletin of the American Physical Society
APS March Meeting 2021
Volume 66, Number 1
Monday–Friday, March 15–19, 2021; Virtual; Time Zone: Central Daylight Time, USA
Session A22: First-Principles Modeling of Excited-State Phenomena in Materials I: Electron-Phonon and Photon-Phonon Interactions
8:00 AM–11:00 AM,
Monday, March 15, 2021
Sponsoring
Units:
DCOMP DCP DMP
Chair: Sahar Sharifzadeh, Boston University
Abstract: A22.00005 : Low-Energy Polaron Spectra in the Doped Fröhlich Model*
9:12 AM–9:24 AM
Live
Presenter:
Nikolaus Kandolf
(ODEN Institute for Computational Engineering and Sciences, University of Texas at Austin)
Authors:
Nikolaus Kandolf
(ODEN Institute for Computational Engineering and Sciences, University of Texas at Austin)
Carla Verdi
(Department of Materials, University of Oxford)
Feliciano Giustino
(ODEN Institute for Computational Engineering and Sciences, University of Texas at Austin)
Fröhlich solid as a model system for electron-phonon coupling in doped polar
semiconductors. Substantial improvements in the resolution of photoemission
spectroscopy have given access to the low-energy physics in these
systems, and have shown that electron-phonon interactions are at the core of a
wide range of intriguing properties, from high electron mobility to superconductivity.
In view of these advances, a sound theoretical description of energy levels and
effective masses in the doped Fröhlich solid is called for. In our study, we present
analytical results for the momentum-resolved spectral function as obtained from the
interacting electron Green’s function. We employ both the first-order
Migdal approximation and the higher-order Cumulant Expansion approach.
We find that the treatment of polaron satellites using the Cumulant Expansion achieves
much better agreement with experiment, albeit at the price of a poorer description of
quasiparticle dispersion relations.
*Work supported as part of the Computational Materials
Sciences Program funded by the U.S. Department of Energy,
Office of Science, Basic Energy Sciences, under Award No.
DE-SC0020129, and by the Robert A. Welch Foundation
under award number F-1990-20190330.
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