Bulletin of the American Physical Society
2024 APS March Meeting
Monday–Friday, March 4–8, 2024; Minneapolis & Virtual
Session Q42: Quantum Materials for Neuromorphic Computing
3:00 PM–5:24 PM,
Wednesday, March 6, 2024
Room: Ballroom B
Sponsoring
Unit:
DCMP
Chair: Javier del Valle, University of Oviedo, Spain
Abstract: Q42.00003 : Imaging Metal-Insulator Patterns in VO2 for Neuromorphic Computing*
4:12 PM–4:48 PM
Presenter:
Alexandre Zimmers
(ESPCI PSL-Sorbonne University)
Author:
Alexandre Zimmers
(ESPCI PSL-Sorbonne University)
(i) How inhomogeneous are these materials? We have developed a new optical microscopy method that allows for the precise sub-micron recording of the insulator-to-metal transition in VO2 neuristors [1]. Using thousands of fully image-stabilized fractal patterns, we have reconstructed and analyzed critical temperature Tc maps and hysteresis width ∆Tc maps.
(ii) What underlying interactions are present? Using image recognition techniques based on a deep learning framework, we have analyzed the entire recorded series of patterns [2]. We find that a two-dimensional Hamiltonian with both nearest neighbor interactions and random field disorder explains the rich spatial structure of the fractal patterns.
(iii) Can critical temperature maps be engineered? Recently, ramp-reversal temperature sweeps have been reported to change the transition temperature in these materials. By optically tracking the fractal patterns, Tc change is shown to occur deep inside both insulating and metallic clusters throughout the entire sample. We find that a theoretical model of the diffusion of point defects for the observed changes and subsequent erasing over the entire sample surface [3].
[1] arXiv:2301.04220 (2023)
[2] Phys.Rev.B 107, 205121 (2023)
[3] Adv. Electron. Mater. 2023, 9, 2300085 (2023)
*European Union's Horizon 2020 - Marie Skłodowska-Curie Grant no. 945304. NSF DMR-2006192, IIP-1827536, DMR-2011738. NSF XSEDE Grants No. TG-DMR-180098 and DMR-190014. HEERF III (ARP) P425F204928. DOE BES DE-SC0022277. FA9550-20-1-0242.
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