Possible surface magnetism in the topological Kondo insulator candidate FeSi*

Our group has previously reported the existence of a conducting surface state (CSS) in FeSi, a candidate for a d-electron topological Kondo insulator (TKI), at low temperature. In this work, we present the electrical transport properties of single crystals of FeSi studied in the phase space of temperature (T), magnetic field (B), and the angle (θ) between the electrical current and B. The normalized T-dependent electrical resistance (R) of a successively thinned FeSi crystal provides further confirmation of the existence of a CSS. We report that in the CSS, the magnetoresistance (MR) exhibits a hysteresis loop bounded within ± 0.5 T, suggesting two-dimensional magnetic ordering. The hysteretic MR is asymmetric in B and anisotropic with respect to θ. Further exploration of R(θ) at a fixed field of 9 T reveals an initial progressive rotation of the axis for two-fold rotational symmetry from 2 K to 10 K, then a stabilized axis for two-fold symmetry until at T > 40 K, the anisotropy vanishes, coincident with the disappearance of the CSS. These observations point to a possible magnetically ordered surface state that has been reported in similar systems such as FeSi nanofilms and bulk SmB₆.