Magnetotransport studies in hybrid 2D/0D nanostructures*

We present a device fabrication strategy that takes advantage of stacking techniques developed for van der Waals heterostructures to construct hybrid 2D/0D composite nanostructures, with potential application in the study of spin and charge disorder as well as magnetic-proximity effects. The structures in this study are comprised of superparamagnetic iron oxide nanoparticles (SPIONs) and monolayer graphene. The SPIONs are deposited first using a Langmuir-Blodgett technique, yielding rafts of highly ordered nanoparticles. Characterization via magnetic force microscopy (MFM) reveals magnetic order at multiple length scales and SQUID magnetometry identifies both glassy antiferromagnetic and ferromagnetic response. Single graphene monolayers are mechanically stacked on the SPION layer, and are found to maintain relatively high mobility and gate sensitivity, as indicated by quantum Hall effect (QHE) measurements.